It does once you're used to 60fps. Playing Gotham just wasn't smooth, fluid or responsive. I think it also depends on the type of game. Requiem at 40fps with VRR on my LG CX OLED plays and feels better but it's a slow paced stealth oriented game with some chase/action scenes where as Gotham, there's a lot of combat and it needs that fluidity that it's simply lacking.
Last generation, games at 30fps like HZD or GOW and others felt great because the combat/gameplay itself was great. A game like Gotham where it's not great just becomes worse at 30fps where as with 60fps, it would help out the game to feel better to play.
Sure, better looking games are welcome but in all honesty, the only game this generation that I could say I was disappointed in regards to visuals was Halo Infinite but the combat/gameplay at 60fps made up for it and is an exchange I will always take regardless of the game.
I just wish the developers and publishers would concentrate on the performance aspects of their games and at the very least, just give me the option for 60fps even if it's at 1080p since im not a resolution or visuals guy.